The author presents a fully ab initio scheme to model transient spectroscopy signals in the presence of strongly bound excitons. Using LiF as a prototype material, the authors shows that the scheme is able to capture the exciton signature both in time-resolved angle-resolved photoemission spectroscopy and transient absorption experiments. The approach is completely general and can become the reference scheme for modeling pump and probe experiment in a wide range of materials.

D. Sangalli Phys. Rev. Materials 5, 083803

Type of paper:

The author presents a fully ab initio scheme to model transient spectroscopy signals in the presence of strongly bound excitons. http://arxiv.org/abs/2106.03592

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https://doi.org/10.1103/PhysRevMaterials.5.083803